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Mercury dynamics and mass balance in a subtropical forest, southwestern China

文献类型: 外文期刊

作者: Ma, Ming 1 ; Wang, Dingyong 1 ; Du, Hongxia 1 ; Sun, Tao 1 ; Zhao, Zheng 1 ; Wang, Yongmin 1 ; Wei, Shiqiang 1 ;

作者机构: 1.Southwest Univ, Coll Resources & Environm, Chongqing 400715, Peoples R China

2.Chongqing Key Lab Agr Resources & Environm, Chongqing 400715, Peoples R China

期刊名称:ATMOSPHERIC CHEMISTRY AND PHYSICS ( 影响因子:5.2; 五年影响因子:5.7 )

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收录情况: SCI

摘要: The mid-subtropical forest area in southwest China was affected by anthropogenic mercury (Hg) emissions over the past 3aEuro-decades. We quantified mercury dynamics on the forest field and measured fluxes and pools of Hg in litterfall, throughfall, stream water and forest soil in an evergreen broadleaved forest field in southwestern China. Total Hg (THg) input by the throughfall and litterfall was assessed at 32.2 and 42.9aEuro-A mu gaEuro-m(-2)aEuro-yr(-1), respectively, which was remarkably higher than those observed from other forest fields in the background of North America and Europe. Hg fluxes across the soil-air interface (18.6aEuro-mgaEuro-m(-2)aEuro-yr(-1)) and runoff and/or stream flow (7.2aEuro-A mu gaEuro-m(-2)aEuro-yr(-1)) were regarded as the dominant ways for THg export from the forest field. The forest field hosts an enormous amount of atmospheric Hg, and its reserves is estimated to be 25aEuro-341aEuro-A mu gaEuro-m(2). The ratio of output to input Hg fluxes (0.34) is higher compared with other study sites. The higher outputaEuro-/aEuro-input ratio may represent an important ecological risk for the downstream aquatic ecosystems, even if the forest field could be an effective sink of Hg.

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