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Atmospheric mercury deposition and its contribution of the regional atmospheric transport to mercury pollution at a national forest nature reserve, southwest China

文献类型： 外文期刊

作者： Ma, Ming 1 ; Wang, Dingyong 1 ; Du, Hongxia 1 ; Sun, Tao 1 ; Zhao, Zheng 1 ; Wei, Shiqing 1 ;

作者机构： 1.Southwest Univ, Coll Resource & Environm, Minist Educ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Chongqing 400715, Peoples R China

2.Chongqing Key Lab Agr Resources & Environm, Chongqing 400716, Peoples R China

关键词： Mercury;Subtropical forest;Deposition fluxes;Gaseous elemental mercury;Source

期刊名称：ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH （ 影响因子：4.223； 五年影响因子：4.306 ）

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收录情况： SCI

摘要： Atmospheric mercury deposition by wet and dry processes contributes to the transformation of mercury from atmosphere to terrestrial and aquatic systems. Factors influencing the amount of mercury deposited to subtropical forests were identified in this study. Throughfall and open field precipitation samples were collected in 2012 and 2013 using precipitation collectors from forest sites located across Mt. Jinyun in southwest China. Samples were collected approximately every 2 weeks and analyzed for total (THg) and methyl mercury (MeHg). Forest canopy was the primary factor on THg and MeHg deposition. Simultaneously, continuous measurements of atmospheric gaseous elemental mercury (GEM) were carried out from March 2012 to February 2013 at the summit of Mt. Jinyun. Atmospheric GEM concentrations averaged 3.8 +/- 1.5 ng m(-3), which was elevated compared with global background values. Sources identification indicated that both regional industrial emissions and long-range transport of Hg from central, northeast, and southwest China were corresponded to the elevated GEM levels. Precipitation deposition fluxes of THg and MeHg in Mt. Jinyun were slightly higher than those reported in Europe and North America, whereas total fluxes of MeHg and THg under forest canopy on Mt. Jiuyun were 3 and 2.9 times of the fluxes of THg in wet deposition in the open. Highly elevated litterfall deposition fluxes suggest that even in remote forest areas of China, deposition of atmospheric Hg-0 via uptake by vegetation leaf may be a major pathway for the deposition of atmospheric Hg. The result illustrates that areas with greater atmospheric pollution can be expected to have greater fluxes of Hg to soils via throughfall and litterfall.

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